— |- | scope="row" | "Older and Bolder"b/w "I'd Trade All of My Tomorrows (For Just One Yesterday)" | 3 | — |- | scope="row" | "I Want to Thank You Lord"b/w "My Desire" | — | — |- | scope="row" | "Eddy's Song"b/w "Condemned Without Trial" | 1 | — | align="left"| Eddy's Songs|- | rowspan="7"| 1953 | scope="row" | "I’m Gonna Sit Right Down (And Write Myself a Letter)"b/w "I’m Waiting for the Ships That Never Come In" | — | — | align="left" rowspan="4"| All-Time Favorites|- | scope="row" | "When Your Hair Has Turned to Silver"b/w "Angry" | — | — |- | scope="row" | "Moonlight and Roses (Bring Mem'ries of You)"b/w "The Missouri Waltz" | — | — |- | scope="row" | "I’m Gonna Lock My Heart"b/w "You Always Hurt the One You Love" | — | — |- | scope="row" | "Free Home Demonstration"b/w "How's the World Treating You" (z albumu You Gotta Have Love) | 4 | — | align="left" rowspan="2"|utwory spoza albumu |- | scope="row" | "Mama, Come Get Your Baby Boy"b/w "If I Never Get to Heaven" (z albumu Let's Make Memories Tonight) | 4 | — |- | scope="row" | "I Really Don’t Want to Know"b/w "I'll Never Get Over You" (utwór spoza albumu) | 1 | — | align="left"|Eddy Arnold Sings Them Again|- | rowspan="5"| 1954 | scope="row" | "Robe of Calvary"b/w "Prayer" | — | — | align="left" rowspan="2"|The Chapel on the Hill|- | scope="row" | "The Chapel on the